The Influence of Long-range Transport on Springtime Nocturnal Ozone Enhancement in Seoul

봄철 서울지역 야간 오존농도 상승에 미치는 장거리 수송의 영향

  • Published : 2004.08.01

Abstract

In Seoul metropolitan area, nocturnal variation of surface ozone concentrations observed at 27 monitoring sites from 1998 to 2002 showed that high ozone levels occurred frequently during the spring. Frequency distributions for nighttime ozone indicated that elevated concentrations in spring were influenced by advection of different air mass compared to other seasons. Surface wind analysis during the spring revealed that relatively strong southwesterly winds were associated with nocturnal ozone enhancement, which can be attributed to the regional transport of ozone. In order to identify the origin of nocturnal ozone enhancement in spring, 3-day backward trajectories were calculated by HYSPLIT 4 for the episode days and then classified. The results showed that NW, W, and SW flows, indicating influence of polluted air masses from the China continent, have 51% in a]1 the episode days, which suggest that the nocturnal ozone enhancement can occur under the effect of long-range transport of ozone-laden air mass on a regional scale. Case study of nocturnal ozone maxima associated with long-range transport was discussed in more detail in the light of meteorological conditions. Southwesterly synoptic flow along the outer edge of moving high-pressure system was found to be the important cause of nocturnal ozone maxima in Seoul. This flow could lead to be long-range transport of ozone that had effectively accumulated in the stagnating portion of the system located eastern coast of China. Low atmosphere soundings, backward trajectories, and elevated ozone and CO levels at the back-ground tiles gave evidence for regional effects on nocturnal ozone enhancement In Seoul.

Keywords

References

  1. 한국대기보전학지 v.12 no.1 고산에서의 1994년 3~4월 측정연구:(II) 기체상 대기오염물질의 특성 김용표;김진영;박세옥;김성주;심상규;문길주;박경윤;허철구
  2. 한국기상학회지 v.36 no.2 서울.인천지역 자동기상관측 바람 자료의 특성 분석 김진영;김영성;정관영
  3. 대기환경연보(2001) 환경부
  4. J. Geophys. Res. v.101 Long range transport of ozone in the East Asian Pacific rim region Akimoto, H.;H. Mukai;M. Nishikawa;K. Murano;S. Hatakeyama;C.M. Liu;M. Buhr;K.J. Hsu;D.A. Jaffe;L. Zhang;R. Honrath;J.T. Merrill;R.E. Newell https://doi.org/10.1029/95JD00025
  5. Atmos. Environ. v.33 Experimental determination of the effect of mountain-valley breeze circulation on air pollution in the vicinity of Freiburg Baumbach, G.;U. Vogt
  6. J. Geophys. Res. v.103 no.D9 Tropospheric ozone production and transport in the springtime in east Aisa Carmichael, G.R.;I. Uno,M.J. Phadnis;Y. Zhang;Y. Sunwoo https://doi.org/10.1029/97JD03740
  7. J. Geophys. Res. v.105 The effect of meteorology and air pollution transport on ozone episodes at a subtropical coastal Asian city, Hong Kong Chan, C.Y.;L.Y. Chan https://doi.org/10.1029/2000JD900140
  8. J. Geophys. Res. v.105 Meterological controls on ozone at an elevated eastern United States regional background monitoring site Cooper, O.R.;J.L. Moody
  9. Atmos. Environ. v.31 no.13 Ozone concentration jump in the stable nocturnal boundary layer during a LLJ-event Corsmeier, U.;N. Kalthoff;O. Kolle;M. Kotzian;F. Fiedler https://doi.org/10.1016/S1352-2310(96)00358-5
  10. Atmos. Environ. v.37 no.13 Summer nocturnal ozone maxima in Goteborg, Sweden Eliasson, I.;S. Thorsson;A.S. Yvonne https://doi.org/10.1016/S1352-2310(03)00205-X
  11. Air & Waste Manage. Assoc. v.44 Ground-level ozone in eastern Canada: seasonal variations, trends, and occurrences of high concentrations Fuentes, J.D.;T.F. Dann https://doi.org/10.1080/10473289.1994.10467296
  12. J. Geophys. Res. v.105 Characteristics of groundlevel ozone distributions in Korea for the period of 1990~1995 Ghim, Y.S.;Y.S. Chang https://doi.org/10.1029/1999JD901179
  13. Atmos. Environ. v.37 Six 'new' episodes of trans-Pacific transport of air pollutants Jaffe, D.;I. McKendry;T. Anderson;H. Price https://doi.org/10.1016/S1352-2310(02)00862-2
  14. Proceeding of the 8th International conference on ASAAQ Seasonal characteristics of surface ozone associated with flow patterns at Kanghwa back-ground monitoring site in the western Korea Kim, Y.K.;H.W. Lee;I.B. Oh;Y.S. Moon;S.K. Song
  15. Atmos. Environ. v.35 Flow patterns influencing the seasonal behavior of surface ozone and carbon nomoxide at a coastal site near Hong Kong Lam, K.S.;T.J. Wang;L.Y. Chan;T. Wang;J. Harris https://doi.org/10.1016/S1352-2310(00)00559-8
  16. Atmos. Environ. v.36 Ozone episodes in urban Hong Kong 1994~1999 Lee, Y.C.;G. Calori, G.;Hills, P.;G.R. Carmichael https://doi.org/10.1016/S1352-2310(02)00150-4
  17. Atmos. Environ. v.24A A study of Taipei ozone problem Liu, C.M.;S.C. Liu;S.H. Shen
  18. an assessment of tropospheric ozone pollution-a North American perspective, C3-34 NARSTO(North American Research Strategy for Tropospheric Ozone)
  19. J. Geophys. Res. v.105 Mixing of anthropogenic pollution with stratospheric ozone: A case study from the North Atlantic wintertime troposphere Parrish, D.D.;J.S. Holloway;R. Jakoubek;M. Trainer;T.B. Ryerson;G. Hubler;F.C. Fehsenfeld https://doi.org/10.1029/2000JD900291
  20. Atmos. Environ. v.36 Surface ozone at four remote island sites ad the preliminary assessment of the exceedances of its critical level in Janpan Pochanart, P.;H. Akimoto;Y. Kinjo;H. Tanimoto https://doi.org/10.1016/S1352-2310(02)00339-4
  21. J. Geophys. Res. v.103 Influence of regional-scale anthropogenic activity in northeast Asia on seasonal variations of surface ozone and caron monoxide observed Oki, Japan Pochanart, P.;J. Hirokawa;Y. Kajii;H. Akimoto
  22. Atmos. Environ. v.34 Nocturnal secondary ozone concentration maxima analysed by sodar observations and surface measurements Reitebuch, O.;A. Strassburger;S. Emeis;W. Kuttler https://doi.org/10.1016/S1352-2310(00)00185-0
  23. Atmos. Environ. v.36 Secondary ozone maxima in a very stable nocturnal boundary layer: observations from the Lower Fraser Valley, BC Salmond, J.A.;I.G. McKendry https://doi.org/10.1016/S1352-2310(02)00698-2
  24. Atmos. Environ. v.12 Nocturnal ozone maxima Samson, P.J. https://doi.org/10.1016/0004-6981(78)90035-5
  25. Atmos. Environ. v.34 Present and future emissions of air pollutants in China: SO$_2$, NOx and CO Streets, D.G.;S.T. Waldhoff https://doi.org/10.1016/S1352-2310(99)00167-3
  26. J. Appl. Met. v.27 Flow mechanism for the long-range transport air pollutants by the sea breeze causing inland nighttime high oxidants Ueda, H.;S. Mitsumoto;H. Kurita https://doi.org/10.1175/1520-0450(1988)027<0182:FMFTLR>2.0.CO;2
  27. Atmos. Environ. v.35 A study of surface ozone and the relation to complex wind flow in Hong Kong Wang, T.;Y.Y. Wu;T.F. Cheung;K.S. Lam https://doi.org/10.1016/S1352-2310(00)00558-6
  28. Atmos. Environ. v.23 Parameterization of surface resistance to gaseous dry deposition in regional scale numerical models Wesely, M.L. https://doi.org/10.1016/0004-6981(89)90153-4
  29. Atmos. Environ. v.35 A study of surface ozone and the relation to complex wind flow in Hong Kong Wang, T.;Y.Y. Wu;T.F. Cheung;K.S. Lam https://doi.org/10.1016/S1352-2310(00)00558-6
  30. Atmos. Environ. v.23 Parameterization of surface resistance to gaseous dry deposition in regional scale numerical models Wesely, M.L. https://doi.org/10.1016/0004-6981(89)90153-4