Analysis of Metabolism and Effective Half-life for Tritium Intake of Radiation Workers at Pressurized Heavy Water Reactor

중수로원전 종사자의 삼중수소 체내섭취에 따른 인체대사모델과 유효반감기 분석

  • Published : 2009.06.30

Abstract

Tritium is the one of the dominant contributors to the internal radiation exposure of workers at pressurized heavy water reactors (PHWRs). This nuclide is likely to release to work places as tritiated water vapor (HTO) from a nuclear reactor and gets relatively easily into the body of workers by inhalation. Inhaled tritium usually reaches the equilibrium of concentration after approximately 2 hours inside the body and then is excreted from the body with a half-life of 10 days. Because tritium inside the body transports with body fluids, a whole body receives radiation exposure. Internal radiation exposure at PHWRs accounts for approximately 20-40% of total radiation exposure; most internal radiation exposure is attributed to tritium. Thus, tritium is an important nuclide to be necessarily monitored for the radiation management safety. In this paper, metabolism for tritium is established using its excretion rate results in urine samples of workers at PHWRs and an effective half-life, a key parameter to estimate the radiation exposure, was derived from these results. As a result, it was found that the effective half-life for workers at Korean nuclear power plants is shorter than that of International Commission on Radiological Protection guides, a half-life of 10 days.

삼중수소는 중수로형 원전에서 방사선작업종사자의 내부피폭을 일으키는 주요 방사성핵종 중의 하나이다. 이 핵종은 계통에서 HTO 형태로 비교적 쉽게 누설되며, 호흡과정을 통해 작업종사자의 신체내부로 유입된다. 이러한 삼중수소는 신체 내에서 약 2시간 후에 평형에 도달하며, 약 10일의 유효반감기를 가지고 신체로부터 제거된다. 신체내의 삼중수소는 체액을 따라 유동하기 때문에 전신이 피폭을 받게 된다. 원전의 운영경험에 의하면 원전종사자의 전체 피폭방사선량의 약 20$\sim$40% 정도가 삼중수소에 의한 내부피폭으로 발생하고 있다. 따라서, 원전의 방사선안전관리 측면에서 볼 때 중요하게 관리되는 방사성핵종이다. 본 논문에서는 중수로 원전에서 삼중수소의 흡입에 따른 뇨시료 중의 삼중수소 방사능 측정 자료를 이용하여 삼중수소의 인체 대사모델을 수립하고, 이를 근거로 피폭방사선량 평가의 중요 인자인 유효반감기를 분석하였다. 이 결과에 따르면 국내 원전 종사자의 유효반감기는 국제방사선 방호위원회에서 제시한 10일보다 짧은 것으로 나타났다.

Keywords

References

  1. 원자력발전소 방사선 관리 연보. 2007
  2. Whillans DW, Thind KS. Internal Dosimetry for Short- Range Emitters. Health Physics Society 1995 Summer School (Radiation Protection at Nuclear Reactors). Medical Physics Publishing Madison, Wisconsin. 1995
  3. Wolodarsky B. OPG Tritium Dosimetry. Radiation Protection Workshop. 2005
  4. 한국수력원자력(주). 원자력발전소주변 환경방사선 조사보고서.2007
  5. Ontario Power Generation. Annual Summary and Assessment of Environmental Radiological Data for 2005. N-REP-03481-10004-R01. 2006
  6. Canadian Standards Association. Guidelines for Calculating Derived Release Limits for Radioactive material in Airborne and Liquid Effluents for Normal Operation of Nuclear Facilities. CAN/CSA-N288.1-M87. 1987
  7. International Atomic Energy Agency, Methods for Assessing Occupational Radiation Doses Due to Intakes of Radionuclides. Safety Report Series No. 37, 2004
  8. Atomic Energy Control Board. Regulatory Document R- 100; The Determination of Effective Doses from the Intake of Tritiated Water. 1987
  9. 교육과학기술부. 고시 제 2008-51호;내부피폭 방사선량의 측정 및 산출에 관한 규정,2009
  10. International Commission on Radiation Protection. Individual Monitoring for Internal Exposure of Workers. Replacement of ICRP-54. ICRP Publication 78. Pergamon Press. 1997
  11. National Council on Radiation Protection and Measurement. Tritium and Other Radionuclide Labelled Organic Compounds Incorporated in Genetic Materials. NCRP-63. 1979
  12. Hill RL, Johnson JR. Metabolism and Dosimetry of Tritium. Health Physics. 1993;65(6):628-647 https://doi.org/10.1097/00004032-199312000-00003
  13. International Commission on Radiation Protection. Limits for intakes of radionuclides by workers. ICRP Publication 30. New York: Pergamon Press. 1982
  14. Okada S, Momoshima N. Overview of tritium: Characteristics, sources and problems. Health Physics. 1993;65(6):595-609 https://doi.org/10.1097/00004032-199312000-00001
  15. Wong KY, Khan TA, Guglelmi F, Kvetton OK, Macphee RC. Canadian tritium experience. Canadian Fusion Fuels Technology Project, Toronto, Ontario, Canada. 1984
  16. Balonov MI, Dolgirev EI, Likhtarev IA. Exchange kinetics and dosimetry of tritium oxide in man for different routes of administration. Health Physics. 1974;27:367-375 https://doi.org/10.1097/00004032-197410000-00005
  17. Bush WR. AECL-4150; Assessing and controlling the hazard from tritiated water, Atomic Energy of Canada Limited, Chalk River, Canada. 1972
  18. Taylor DM, Moroni JP, Snihs JO, Richmond CR. The Metabolism of H-3 and C-14 with Special Reference to Radiation Protection. Radiat. Protect. Dosim. 1990;30:87-93 https://doi.org/10.1093/oxfordjournals.rpd.a080603
  19. Butler HL, Leroy JH. Observation of the Biological Halflife of Tritium. Health Physics. 1965;11:283-290 https://doi.org/10.1097/00004032-196504000-00005
  20. Etnier EL, Travis CC, Hetrick DM. Metabolism of Organically Bound Tritium in Man. Radiat. Res. 1984;100:487-502 https://doi.org/10.2307/3576412
  21. Dunford DW, Johnson JR. AECL-9434; GENMOD-A Program for Internal Dosimetry Calculation. 1987
  22. 이형석, 김위수, 김희근, 김은주, 양양희, 중수로원전에서 발생하는 삼중수소 및 C-14의 작업자 선량평가를 위한 인체대사모델 연구, 한국원자력학회추계학술대회, 2002.10.24, 2002
  23. 김희근, 김용배,김위수, 김은주, 이형석.상중수소 인체대사모델 및 유효반감기 검토, 대한방사선방어학회 춘계학술대회, 2001.4.27, 2001
  24. 한국수력원자력(주).원자력발전소 표준기술행정 절차서;내부피폭 방사선량의 측정 및 평가, 표준기 행 방사선 -06.2003
  25. 교육과학기술부.중수로 원전 운전 안전성 현안연구(최종보고서).2002