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Analysis of PM2.5 Case Study Burden at Chungju City

충주시 미세입자 (PM2.5) 농도특성에 대한 사례 연구

  • Lee, Sung-Hee (Department of Environmental Engineering, Korea National University of Transportation) ;
  • Kang, Byung-Wook (Department of Environmental Engineering, Korea National University of Transportation) ;
  • Yeon, Ik-Jun (Department of Environmental Engineering, Korea National University of Transportation) ;
  • Choi, Jun-Rack (Department of Environmental Engineering, Korea National University of Transportation) ;
  • Park, Hyun-Pill (Department of Environmental Engineering, Korea National University of Transportation) ;
  • Park, Sang-Chan (Department of Environmental, Civil and Information System, Seowon University) ;
  • Lee, Hak Sung (Department of Environmental, Civil and Information System, Seowon University) ;
  • Cho, Byung-Yeol (Department of Environmental Engineering, Korea National University of Transportation)
  • 이성희 (한국교통대학교 환경공학과) ;
  • 강병욱 (한국교통대학교 환경공학과) ;
  • 연익준 (한국교통대학교 환경공학과) ;
  • 최준락 (한국교통대학교 환경공학과) ;
  • 박현필 (한국교통대학교 환경공학과) ;
  • 박상찬 (서원대학교 환경건설정보학과) ;
  • 이학성 (서원대학교 환경건설정보학과) ;
  • 조병렬 (한국교통대학교 환경공학과)
  • Received : 2012.07.11
  • Accepted : 2012.09.27
  • Published : 2012.10.31

Abstract

Fine particles ($PM_{2.5}$) were collected and analyzed from April 2010 through January 2011 in Chungju to investigate the characteristics of $PM_{2.5}$ and its ionic species. The annual mean concentrations of $PM_{2.5}$, ${SO_4}^{2-}$, $NO_3{^-}$, and $NH_4{^+}$ in the particulate phase were 40.84, 7.61, 7.14 and $3.74{\mu}g/m^3$, respectively. $PM_{2.5}$ concentrations were higher in fall and spring than in winter and summer. The elevated concentrations episodes are the main factor that enhanced the $PM_{2.5}$ concentrations in the fall. Among the major ionic species ${SO_4}^{2-}$ showed the highest concentration, followed by $NO_3{^-}$ and $NH_4{^+}$, $NO_3^-$ exhibited higher concentrations during the winter, but ${SO_4}^{2-}$ and $NH_4{^+}$ were not showed seasonal variation. The high correlations were found among $PM_{2.5}$, ${SO_4}^{2-}$, $NO_3{^-}$ and $NH_4{^+}$ during all seasons except for spring. The evaluation of backward trajectories and meteorological records show that the highest $PM_{2.5}$ concentration levels occurred during W-NW weather conditions, which influenced by the emission sources of China area. The low pollution levels generally occurred during E-S weather conditions, which influenced by the East Sea and south of the Yellow Sea. The elevated $PM_{2.5}$ mass concentrations arouse the concentration of $NO_3{^-}$, but no effects on ${SO_4}^{2-}$ and $NH_4{^+}$.

Keywords

References

  1. Barblaux, M., P.A. Scheff, and L.R. Babcock (1992) Characterization of respirable particulate matter in Mexico city, Mexico, Presentation at the 9th World Clean Air Congress and Exhibition, Montreal, Canada, August 30-September 4, IU-7.07.
  2. Bari, A., V.A. Dutkiewicz, C.D. Judd, L.R. Wilson, D. Luttinger, and L. Husain (2003) Regional sources of particulate sulfate, $SO_{2}$, $PM_{2.5}$, HCl, and $HNO_{3}$ in New York, NY, Atmospheric Environment, 37, 2837- 2844. https://doi.org/10.1016/S1352-2310(03)00200-0
  3. Brook, J.R., A.H. Wiebe, S.A. Woodhouse, C.V. Audette, T.F. Dann, S. Callaghan, M. Piechowski, E. Dabek-Zlotorzynska, and J.F. Dloughy (1997) Temporal and spatial relationships in fine particle strong acidity, sulfhate, $PM_{10}$, and $PM_{2.5}$ across multiple Canadian locations, Atmospheric Environment, 31(24), 4223- 4236. https://doi.org/10.1016/S1352-2310(97)00248-3
  4. Choi, M.-K., H.-G. Yeo, J.E. Lim, K.-C. Cho, and H.-K. Kim (2000) Characteristics of $PM_{2.5}$ in Kangwha, J. KOSAE, 16(6), 573-583. (in Korean with English abstract)
  5. Dockery, D.W. and C.A. Pope III (1994) Acute respiratory effects of particulate air pollution, Annu. Rev. Public. Health, 15, 107-132. https://doi.org/10.1146/annurev.pu.15.050194.000543
  6. Dockery, D.W., C.A. Pope III, X. Xu, J.D. Spengler, J.H. Ware, and M.E. Fay (1993) An association between air pollution and mortality in six U.S. Cities, N. Engl. J. Med., 329, 1753-1759. https://doi.org/10.1056/NEJM199312093292401
  7. Dockery, D.W., J. Schwartz, and J.D. Spengler (1992) Air pollution and daily mortality: Associations with particulates and acid aerosols, Environ. Res., 59, 362-373. https://doi.org/10.1016/S0013-9351(05)80042-8
  8. Gomiscek, B., A. Frank, H. Puxbaum, S. Stopper, O. Preining, and H. Hauck (2004) Case study analysis of PM burden at an urban and a rural site during the AUPHEP project, Atmos. Environ., 38, 3935-3948. https://doi.org/10.1016/j.atmosenv.2004.03.033
  9. He, K., F. Yang, Y. Ma, Q. Zhang, X. Yao, C.K. Chan, S. Cadle, T. Chan, and P. Mulawa (2001) The characteristics of $PM_{2.5}$ in Beijing, China, Atmos. Environ., 35, 4959-4970. https://doi.org/10.1016/S1352-2310(01)00301-6
  10. Hwang, G.-Y., M.-H. Lee, B.-C. Shin, G.-W. Lee, J.-H. Lee, and J.-S. Shim (2008) Mass concentration and ionic composition of $PM_{2.5}$ observed at Ioedo ocean research station, J. KOSAE, 24(5), 501-511. (in Korean with English abstract) https://doi.org/10.5572/KOSAE.2008.24.5.501
  11. Jung, J.-H. and Y.-J. Han (2008) Study on characteristics of PM2.5 and its ionic constituents in Chuncheon, Korea, J. KOSAE, 24(6), 682-692. (in Korean with English abstract)
  12. Kang, B.-W., H.S. Lee, and H.-K. Kim (1997) A seasonal variation of acidic gases and fine particle species in Chongju area, J. KOSAE, 13(5), 333-343. (in Korean with English abstract)
  13. Kang, C.-H., W.-H. Kim, J.-S. Han, Y. Sunwoo, and K.-C. Moon (2003) Pollution characteristics of $PM_{2.5}$ fine particles collected at Gosan site in Jeju island during 1997-2001, J. KOSAE, 19(3), 263-273. (in Korean with English abstract)
  14. Kang, C.-M., B.-W. Kang, and H.S. Lee (2006) Source identification and trends in concentrations of gaseous and fine particulate principal species in Seoul, South Korea, J. Air & Waste Manage. Assoc., 56, 911-921. https://doi.org/10.1080/10473289.2006.10464506
  15. Klemm, R.J., R.M. Mason Jr., C.M. Heilig, L.M. Neas, and D.W. Dockery (2000) Is daily mortality associated specifically with fine particles? Data reconstruction and replication of analyses, J. Air Waste Manag. Assoc., 50, 1215-1222. https://doi.org/10.1080/10473289.2000.10464149
  16. Lee, H.S., R.A. Wadden, and P.A. Scheff (1993) Measurement and evaluation of acid air pollutants in Chicago using an annular denuder system, Atmos. Environ., 27A(4), 543-553.
  17. Lee, H.W., T.-J. Lee, and D.-S. Kim (2009) Identifying ambient PM2.5 sources and estimating their contributions by using PMF: separation of gasoline and diesel automobile sources by analyzing ECs and OCs, J. KOSAE, 25(1), 75-89. (in Korean with English abstract) https://doi.org/10.5572/KOSAE.2009.25.1.075
  18. Liabaca, M., I. Olaeta, E. Campos, J. Villaire, M. Tellez-Rojo, and I. Romieu (1999) Association between levels of fine particulate and emergency visits for pneumonia and other respiratory illnesses among children in Satiago, Chile, J. Air Waste Manag. Assoc., 49, 154- 163. https://doi.org/10.1080/10473289.1999.10463879
  19. Lighty, J.S., J.M. Veranth, and A.F. Sarofim (2000) Combustion aerosols: Factors governing their size and composition and implications to human health, J. Air Waste Manag. Assoc., 50, 1565-1618. https://doi.org/10.1080/10473289.2000.10464197
  20. Park, J.-S. and S.-D. Kim (2005) The characteristics of secondary carbonaceous species within $PM_{10}$ and $PM_{2.5}$ in Seoul and Incheon area, J. KOSAE, 21(1), 131- 140. (in Korean with English abstract)
  21. Park, S.-C., I.-J. Yeon, B.-R. Cho, J.-S. Cho, and B.-W. Kang (2008) A study on the atmospheric environmental capacity in Chungju area, J. KOSAE, 24(1), 122- 127. (in Korean with English abstract) https://doi.org/10.5572/KOSAE.2008.24.1.122
  22. Schwartz, J. (1996) Air pollution and hospital admissions for respiratory disease, Epidemiology, 7, 20-28. https://doi.org/10.1097/00001648-199601000-00005
  23. U.S. EPA (1989) Determination of reactive acidic and basic gases and particulate matter in indoor air, U.S. Environmental Protection Agency Compendium Chapter IP-9, Atmospheric Research and Exposure Assessment Laboratory, Research Triangle Park, NC.

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