Current Applied Physics

Korean Physical Society (한국물리학회)
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Dielectric, ferroelectric and field-induced strain response of lead-free $BaZrO_3$-modified $Bi_{0.5}Na_{0.5}TiO_3$ ceramics

  • Rahman, Jamil Ur (School of Advanced Material Engineering, Changwon National University) ;
  • Hussain, Ali (School of Advanced Material Engineering, Changwon National University) ;
  • Maqbool, Adnan (School of Advanced Material Engineering, Changwon National University) ;
  • Song, Tae Kwonm (School of Advanced Material Engineering, Changwon National University) ;
  • Kim, Won Jeong (Department of Physics, Changwon National University) ;
  • Kim, Sang Su (Department of Physics, Changwon National University) ;
  • Kim, Myong Ho (School of Advanced Material Engineering, Changwon National University)
  • Received : 2013.06.16
  • Accepted : 2013.12.15
  • Published : 2014.03.31
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Abstract

Lead-free piezoelectric ceramics (1 - x)$Bi_{0.5}Na_{0.5}TiO_3-xBaZrO_3$ (BNT-BZ100x, with x % 0-0.10) were prepared using a conventional solid-state reaction method. The crystal structure, microstructure, dielectric, ferroelectric, and piezoelectric properties of BNTeBZ100x ceramics were studied as functions of different BZ content. X-ray diffraction patterns revealed that the BZ completely diffused in the BNT lattice in the studied composition range. An appropriate amount of BZ addition improved the dielectric, ferroelectric, and piezoelectric properties of BNT ceramics. The remanent polarization (Pr) and piezoelectric constant ($d_{33}$) increased from $22{\mu}C/cm^2$ and 60 pC/N for pure BNT to $30{\mu}C/cm^2$ and 112 pC/N for x % 0.040, respectively. In addition, electric field-induced strain was enhanced to its maximum value ($S_{max}$ % 0.40%) with normalized strain ($d^*{_{33}}$ % $S_{max}/E_{max}$ % 500 pm/V) at an applied electric field of 8 kV/mm for x % 0.055. The enhanced strain can be attributed to the coexistence of ferroelectric and relaxor ferroelectric phases.

Keywords

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