Journal of Korean Society for Atmospheric Environment (한국대기환경학회지)

Korean Society for Atmospheric Environment (한국대기환경학회)
권호 표지
DOI QR코드

DOI QR Code

Source Profile of Road Dust for Statistical Apportionment Modeling in Seoul

통계 수용모델을 위한 서울시 도로변 화학성분 원인 프로파일

  • Park, Da-Jeong (Department of Environmental Engineering, Mokpo National University) ;
  • Han, Young-Ji (Department of Environmental Science, Kangwon National University) ;
  • Lee, Ji-Yi (Department of Environmental Engineering, Chosun University) ;
  • Lee, Kwang-Yul (Department of Environmental Engineering, Gwangju Institute of Science and Technology) ;
  • Cho, In-Hwan (Department of Environmental Engineering, Mokpo National University) ;
  • Park, Eun Ha (Department of Environmental Health, Graduate School of Public Health, Seoul National University) ;
  • Yi, Seung-Muk (Department of Environmental Health, Graduate School of Public Health, Seoul National University) ;
  • Bae, Min-Suk (Department of Environmental Engineering, Mokpo National University)
  • 박다정 (국립목포대학교 환경공학과) ;
  • 한영지 (국립강원대학교 환경과학과) ;
  • 이지이 (조선대학교 환경공학과) ;
  • 이광열 (광주과학기술원 환경공학과) ;
  • 조인환 (국립목포대학교 환경공학과) ;
  • 박은하 (서울대학교 보건대학원 환경보건학과) ;
  • 이승묵 (서울대학교 보건대학원 환경보건학과) ;
  • 배민석 (국립목포대학교 환경공학과)
  • Received : 2015.03.16
  • Accepted : 2015.04.07
  • Published : 2015.04.30
Download PDF
⟨ Previous Next ⟩

Abstract

Sources related to road dust is one of the biggest sources, which is responsible for a large portion of emission. In particular, PM2.5 is a potential cause for respiratory diseases, thus it should be managed and a mitigation plan using results of statistical apportionment modeling such as chemical mass balance needs to be established. Recently, identifying sources of PM2.5 and analyzing the contribution of the road dust through a contribution assessment is required. Therefore, this study provides the chemical source profiles of PM2.5 using IC, GC/MS, OCEC, and XRF for both paved sidewalk and paved roadway collected at seven different sampling sites. As a result, for paved sidewalk, $NH{_4}^+$ (70%), $NO{_3}^-$ (12%), $PO{_4}^-$ (9%), and $SO{_4}^{2-}$ (9%) have been analyzed in PM2.5 mass. Major molecular marker such as Si has been indicated as $12.0{\pm}3.4%$ and $13.6{\pm}6.9%$ for paved sidewalk and roadway, respectively. PAHs such as Fluoranthene, Pyrene, Chrysene, and 1,3,5-Triphenylbenzene are suggested as molecular markers for road dust.

Keywords

References

  1. Adachi, K. and Y. Tainosho (2004) Characterization of heavy metal particles embedded in tire dust, Environ. Int., 30(8), 1009-1017. https://doi.org/10.1016/j.envint.2004.04.004
  2. Amato, F., M. Pandolfi, A. Escrig, X. Querol, A. Alastuey, J. Pey, N. Perez, and P.K. Hopke (2009) Quantifying road dust resuspension in urban environment by Multilinear Engine: A comparison with PMF2, Atmos. Environ., 43(17), 2770-2780. https://doi.org/10.1016/j.atmosenv.2009.02.039
  3. Bae, M.S. and J.J. Schauer (2009) Analysis of Organic Molecular Markers in Atmospheric Fine Particulate Matter: Understanding the Impact of "Unknown" Point Sources on Chemical Mass Balance Models, J. Korean Soc. Atmos. Environ., 25(3), 219-236. (in Korean with English abstract) https://doi.org/10.5572/KOSAE.2009.25.3.219
  4. Bae, M.S., C.H. Jung, Y.S. Ghim, and K.H. Kim (2013) A Proposal for the Upgrade of the Current Operating System of the Seoul's Atmospheric Monitoring Network Based on Statistical Analysis, J. Korean Soc. Atmos. Environ., 29(4), 454-465. (in Korean with English abstract)
  5. Becker, S., J.M. Soukup, and J.E. Gallagher (2002) Differential particulate air pollution induced oxidant stress in human granulocytes, monocytes and alveolar macrophages, Toxicol. in Vitro, 16(3), 209-218. https://doi.org/10.1016/S0887-2333(02)00015-2
  6. Berger, J. and B. Denby (2011) A generalised model for traffic induced road dust emissions. Model description and evaluation, Atmos. Environ., 45(22), 3692-3703. https://doi.org/10.1016/j.atmosenv.2011.04.021
  7. Cadle, S.H., P.A. Mulawa, E.C. Hunsanger, K. Nelson, R.A. Ragazzi, R. Barrett, G.L. Gallagher, D.R. Lawson, K.T. Knapp, and R. Snow (1999) Composition of Light-Duty Motor Vehicle Exhaust Particulate Matter in the Denver, Colorado Area, Environ. Sci. Technol., 33(14), 2328-2339. https://doi.org/10.1021/es9810843
  8. Goel, R. and S.K. Guttikunda (2015) Evolution of on-road vehicle exhaust emissions in Delhi, Atmos. Environ., 105, 78-90. https://doi.org/10.1016/j.atmosenv.2015.01.045
  9. Han, L., G. Zhuang, S. Cheng, Y. Wang, and J. Li (2007) Characteristics of re-suspended road dust and its impact on the atmospheric environment in Beijing, Atmos. Environ., 41, 7485-7499. https://doi.org/10.1016/j.atmosenv.2007.05.044
  10. Han, S.H., J.S. Youn, and Y.W. Jung (2011) Characterization of PM10 and PM2.5 source profiles for resuspended road dust collected using mobile sampling methodology, Atmos. Environ., 45(20), 3343-3351. https://doi.org/10.1016/j.atmosenv.2011.04.015
  11. Harrison, R.M., A.M. Jones, J. Gietl, J. Yin, and D.C. Green (2012) Estimation of the contributions of brake dust, tire wear, and resuspension to nonexhaust traffic particles derived from atmospheric measurements, Environ. Sci. Technol., 46, 6523-6529. https://doi.org/10.1021/es300894r
  12. Kim, W.S. (2010) Characteristics of Particulate Matter by Chemical-Monitoring in Seoul, Korea, Seoul Development Institute Report.
  13. Lee, J.Y., Y.P. Kim, G.N. Bae, S.M. Park, and H.C. Jin (2008) The Characteristics of Particulate PAHs Concentrations at a Roadside in Seoul, J. Korean Soc. Atmos. Environ., 24(2), 133-142. (in Korean with English abstract) https://doi.org/10.5572/KOSAE.2008.24.2.133
  14. Lee, S.B., G.N. Bae, S.M. Park, and S.G. Jung (2007) Black Carbon Pollution Level at a Roadside of Seoul in Spring, J. Korean Soc. Atmos. Environ., 23(4), 466-477. (in Korean with English abstract) https://doi.org/10.5572/KOSAE.2007.23.4.466
  15. Lin, C.C., S.J. Chen, K.L. Huang, W.I. Hwang, G.P. Chang-Chien, and W.Y. Lin (2005) Characteristics of metals in nano/ultrafine/fine/coarse particles collected beside a heavily Trafficked road, Environ. Sci. Technol., 39(21), 8113-8122. https://doi.org/10.1021/es048182a
  16. Park, D.J., J.Y. Ahn, H.J. Shin, and M.S. Bae (2014) Characteristics of PM2.5 Carbonaceous Aerosol, using PILSTOC and GC/MS-TD in Seoul, J. Korean Soc. Atmos. Environ., 30(5), 461-476. (in Korean with English abstract) https://doi.org/10.5572/KOSAE.2014.30.5.461
  17. Peltier, R.E., K.R. Cromar, Y. Ma, Z.H. Fan, and M. Lippmann (2011) Spatial and seasonal distribution of aerosol chemical components in New York City: (2) road dust and other tracers of traffic-generated air pollution, J. of Exposure Sci. Environ. Epidemiol., 21(5), 484-494. https://doi.org/10.1038/jes.2011.15
  18. Schmid, M., S. Zimmermann, H.F. Krug, and B. Sures (2007) Influence of platinum, palladium and rhodium as compared with cadmium, nickel and chromium on cell viability and oxidative stress in human bronchial epithelial cells, Environ. Int., 33(3), 385-390. https://doi.org/10.1016/j.envint.2006.12.003
  19. Woo, D.K., S.B. Lee, G.N. Bae, and T.S. Kim (2008) Comparison of Ultrafine Particles Monitored at a Roadside Using an SMPS and a TR-DMPS, J. Korean Soc. Atmos. Environ., 24(4), 404-414. (in Korean with English abstract) https://doi.org/10.5572/KOSAE.2008.24.4.404

Cited by

  1. Analysis of Poly Aromatic Hydrocarbon (PAH) Pollutants Originated from Local Road Dust by Spacial Measurements vol.32, pp.3, 2016, https://doi.org/10.5572/KOSAE.2016.32.3.272
  2. Comparison of the physical and chemical characteristics of fine road dust at different urban sites vol.68, pp.8, 2018, https://doi.org/10.1080/10962247.2018.1443855